Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit

L. N. Moyes; D. J. Bunker; J. T. Smith; F. R. Livens; C. R. Hughes; J. Hilton; A. Braithwaite; S. Richardson

doi:10.1557/proc-506-757

Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit

L. N. Moyes^*, D. J. Bunker, J. T. Smith, F. R. Livens, C. R. Hughes, J. Hilton, A. Braithwaite, S. Richardson

^*Corresponding author for this work

University of Manchester

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Abstract

Batch sorption experiments have been used to assess the sorption behaviour of four radionuclides, important in the context of low-level waste disposal, on a glacial substrate. Data for sorption of ²³⁸U, ²³⁷Np, ¹³⁴Cs and ⁸⁵Sr are compared and agree well with independent studies. A series of well-established kinetic models have been used to describe the individual uptake mechanisms and rate parameters reported. Sorption occurs via both equilibrium and kinetically controlled pathways, with neptunium sorption being under kinetic control to the greatest extent.

Original language	English
Title of host publication	Materials Research Society Symposium
Subtitle of host publication	Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI
Publisher	Materials Research Society
Pages	[d]757-764
Number of pages	8
DOIs	https://doi.org/10.1557/proc-506-757
Publication status	Published - 1 Dec 1997
Event	Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI - Davos, Switz Duration: 28 Sept 1997 → 3 Oct 1997

Publication series

Name	MRS Online Proceedings Library
Volume	506
ISSN (Print)	1946-4274

Conference

Conference	Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI
City	Davos, Switz
Period	28/09/97 → 3/10/97

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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Moyes, L. N., Bunker, D. J., Smith, J. T., Livens, F. R., Hughes, C. R., Hilton, J., Braithwaite, A., & Richardson, S. (1997). Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit. In Materials Research Society Symposium: Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI (pp. [d]757-764). (MRS Online Proceedings Library; Vol. 506). Materials Research Society. https://doi.org/10.1557/proc-506-757

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title = "Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit",

abstract = "Batch sorption experiments have been used to assess the sorption behaviour of four radionuclides, important in the context of low-level waste disposal, on a glacial substrate. Data for sorption of 238U, 237Np, 134Cs and 85Sr are compared and agree well with independent studies. A series of well-established kinetic models have been used to describe the individual uptake mechanisms and rate parameters reported. Sorption occurs via both equilibrium and kinetically controlled pathways, with neptunium sorption being under kinetic control to the greatest extent.",

author = "Moyes, {L. N.} and Bunker, {D. J.} and Smith, {J. T.} and Livens, {F. R.} and Hughes, {C. R.} and J. Hilton and A. Braithwaite and S. Richardson",

note = "Funding Information: This study was carried out with financial support of British Nuclear Fuels plc.; Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI ; Conference date: 28-09-1997 Through 03-10-1997",

year = "1997",

month = dec,

day = "1",

doi = "10.1557/proc-506-757",

language = "English",

series = "MRS Online Proceedings Library",

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Moyes, LN, Bunker, DJ, Smith, JT, Livens, FR, Hughes, CR, Hilton, J, Braithwaite, A & Richardson, S 1997, Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit. in Materials Research Society Symposium: Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI. MRS Online Proceedings Library, vol. 506, Materials Research Society, pp. [d]757-764, Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI, Davos, Switz, 28/09/97. https://doi.org/10.1557/proc-506-757

Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit. / Moyes, L. N.; Bunker, D. J.; Smith, J. T. et al.
Materials Research Society Symposium: Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI. Materials Research Society, 1997. p. [d]757-764 (MRS Online Proceedings Library; Vol. 506).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

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T1 - Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit

AU - Moyes, L. N.

AU - Bunker, D. J.

AU - Smith, J. T.

AU - Livens, F. R.

AU - Hughes, C. R.

AU - Hilton, J.

AU - Braithwaite, A.

AU - Richardson, S.

N1 - Funding Information: This study was carried out with financial support of British Nuclear Fuels plc.

PY - 1997/12/1

Y1 - 1997/12/1

N2 - Batch sorption experiments have been used to assess the sorption behaviour of four radionuclides, important in the context of low-level waste disposal, on a glacial substrate. Data for sorption of 238U, 237Np, 134Cs and 85Sr are compared and agree well with independent studies. A series of well-established kinetic models have been used to describe the individual uptake mechanisms and rate parameters reported. Sorption occurs via both equilibrium and kinetically controlled pathways, with neptunium sorption being under kinetic control to the greatest extent.

AB - Batch sorption experiments have been used to assess the sorption behaviour of four radionuclides, important in the context of low-level waste disposal, on a glacial substrate. Data for sorption of 238U, 237Np, 134Cs and 85Sr are compared and agree well with independent studies. A series of well-established kinetic models have been used to describe the individual uptake mechanisms and rate parameters reported. Sorption occurs via both equilibrium and kinetically controlled pathways, with neptunium sorption being under kinetic control to the greatest extent.

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M3 - Conference contribution

AN - SCOPUS:0031347756

T3 - MRS Online Proceedings Library

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BT - Materials Research Society Symposium

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Moyes LN, Bunker DJ, Smith JT, Livens FR, Hughes CR, Hilton J et al. Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit. In Materials Research Society Symposium: Proceedings of the 1997 Symposiumon Scientific Basis for Nuclear Waste Management XXI. Materials Research Society. 1997. p. [d]757-764. (MRS Online Proceedings Library). doi: 10.1557/proc-506-757

Sorption kinetics of uranium-238, neptunium-237, caesium-134 and strontium-85 on a glacial deposit

Abstract

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